Versatile electrochemiluminescent biosensor for protein-nucleic acid interaction based on the unique quenching effect of deoxyguanosine-5'-phosphate on electrochemiluminescence of CdTe/ZnS quantum dots.
本文首次报道脱氧鸟苷-5′-磷酸(dGMP)对CdTe/ZnS量子点(QDs)阳极电化学发光(ECL)的高效猝灭效应。该猝灭仅对游离dGMP显著,而不同DNA结构中的dGMP残基几乎不猝灭。作者利用外切酶I(Exo I)从3′到5′方向水解单链DNA并释放dGMP,将dGMP特异性猝灭QDs ECL的现象转化为一种通用生物传感策略,...